Journalartikel

Autorenliste: Müller, MJ; Ziese, F; Belz, J; Hüppe, F; Gowrisankar, S; Bernhardt, B; Schwan, S; Mollenhauer, D; Schreiner, PR; Volz, K; Sanna, S; Chatterjee, S

Jahr der Veröffentlichung: 2022

Seiten: 3517-3529

Zeitschrift: Optical Materials Express

Bandnummer: 12

Heftnummer: 9

ISSN: 2159-3930

Open Access Status: Gold

DOI Link: https://doi.org/10.1364/OME.461427

Verlag: Optica Publishing Group

Abstract: 
Sustainable efficient light emitters based solely on elements-of-hope are needed to replace current compounds based on less-abundant materials. Functionalized diamondoids are a potential solution for this challenge, as a prototypical example offers efficient, octave-spanning emission across the visible spectrum in their single-crystalline form. Its large quantum efficiency increases towards higher-than-ambient temperatures to beyond 7%. The stability beyond 200 degrees C renders such functionalized diamondoids as sustainable phosphors for LED applications. Detailed structural and theoretical investigations suggest a crucial role of exciton states accompanied by structural modifications (self-trapped excitons) in the emission process.

Harvard-Zitierstil: Müller, M., Ziese, F., Belz, J., Hüppe, F., Gowrisankar, S., Bernhardt, B., et al. (2022) Octave-spanning emission across the visible spectrum from single crystalline 1,3,5,7-tetrakis-(p-methoxyphenyl)adamantane, Optical Materials Express, 12(9), pp. 3517-3529. https://doi.org/10.1364/OME.461427

APA-Zitierstil: Müller, M., Ziese, F., Belz, J., Hüppe, F., Gowrisankar, S., Bernhardt, B., Schwan, S., Mollenhauer, D., Schreiner, P., Volz, K., Sanna, S., & Chatterjee, S. (2022). Octave-spanning emission across the visible spectrum from single crystalline 1,3,5,7-tetrakis-(p-methoxyphenyl)adamantane. Optical Materials Express. 12(9), 3517-3529. https://doi.org/10.1364/OME.461427